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Unsubstituted thiophene–diketopyrrolopyrrole conjugated polymer thin films via oxidative chemical vapor deposition – electronic behavior

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cris.lastimport.scopus2024-02-12T20:20:09Z
dc.abstract.enConjugated polymers (CPs) based on diketopyrrolopyrrole (DPP) constitue an important class of high-performance organic semiconductors. While N-alkylation of DPP is required for the solution-based synthesis of DPP-based CPs, oxidative chemical vapour deposition (oCVD) is shown to provide a straightforward solventless and scalable approach for the facile polymerisation of N-unsubstituted DPP. The oCVD reaction of 3,6-di(2-thienyl)-2,5-dihydropyrrolo[3,4-c]pyrrole-1,4-dione (TDPP) yields polymer thin films combining H-bonding and conjugated covalent bonds, resulting in a superior conductivity and a systematic increase of the lifetime of electronically excited states compared to N-alkylated counterparts.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorBoscher, Nicolas D.
dc.contributor.authorZacharias, Helmut
dc.contributor.authorGóra, Monika
dc.contributor.authorKotwica, Kamil
dc.contributor.authorReiker, Tobias
dc.contributor.authorCharyton, Marek K.
dc.date.accessioned2024-01-26T11:19:59Z
dc.date.available2024-01-26T11:19:59Z
dc.date.copyright2023-05-23
dc.date.issued2023
dc.description.accesstimeAT_PUBLICATION
dc.description.financeNie dotyczy
dc.description.number12
dc.description.versionFINAL_PUBLISHED
dc.description.volume4
dc.identifier.doi10.1039/D3MA00197K
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/124247
dc.identifier.weblinkhttp://pubs.rsc.org/en/content/articlepdf/2023/MA/D3MA00197K
dc.languageeng
dc.pbn.affiliationchemical sciences
dc.relation.ispartofMaterials Advances
dc.relation.pages2625-2635
dc.rightsCC-BY
dc.sciencecloudnosend
dc.titleUnsubstituted thiophene–diketopyrrolopyrrole conjugated polymer thin films via oxidative chemical vapor deposition – electronic behavior
dc.typeJournalArticle
dspace.entity.typePublication