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Resilient three-dimensional ordered architectures assembled from nanoparticles by DNA

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cris.lastimport.scopus2024-02-12T19:43:18Z
dc.abstract.enRapid developments of DNA-based assembly methods provide versatile capabilities in organizing nanoparticles (NPs) in three-dimensional (3D) organized nanomaterials, which is important for optics, catalysis, mechanics, and beyond. However, the use of these nanomaterials is often limited by the narrow range of conditions in which DNA lattices are stable. We demonstrate here an approach to creating an inorganic, silica-based replica of 3D periodic DNA-NP structures with different lattice symmetries. The created ordered nanomaterials, through the precise 3D mineralization, maintain the spatial topology of connections between NPs by DNA struts and exhibit a controllable degree of the porosity. The formed silicated DNA-NP lattices exhibit excellent resiliency. They are stable when exposed to extreme temperatures (>1000°C), pressures (8 GPa), and harsh radiation conditions and can be processed by the conventional nanolithography methods. The presented approach allows the use of a DNA assembly strategy to create organized nanomaterials for a broad range of operational conditions.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorMichelson, Aaron
dc.contributor.authorGang, Oleg
dc.contributor.authorMajewski, Paweł
dc.contributor.authorTian, Ye
dc.contributor.authorLiu, Wenyan
dc.contributor.authorStach, Eric A.
dc.contributor.authorYager, Kevin G.
dc.contributor.authorCordeiro, Marco A. L.
dc.contributor.authorTian, Cheng
dc.contributor.authorMa, Chunli
dc.contributor.authorKisslinger, Kim
dc.date.accessioned2024-01-25T19:13:26Z
dc.date.available2024-01-25T19:13:26Z
dc.date.copyright2021-03-19
dc.date.issued2021
dc.description.accesstimeAT_PUBLICATION
dc.description.financePublikacja bezkosztowa
dc.description.number12
dc.description.versionFINAL_PUBLISHED
dc.description.volume7
dc.identifier.doi10.1126/SCIADV.ABF0617
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/118471
dc.identifier.weblinkhttps://syndication.highwire.org/content/doi/10.1126/sciadv.abf0617
dc.languageeng
dc.pbn.affiliationchemical sciences
dc.relation.ispartofScience Advances
dc.rightsCC-BY-NC
dc.sciencecloudnosend
dc.titleResilient three-dimensional ordered architectures assembled from nanoparticles by DNA
dc.typeJournalArticle
dspace.entity.typePublication