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Controlling magnetic exchange and anisotropy by nonmagnetic ligand substitution in layered MPX3 (M=Ni, Mn; X=S, Se)

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dc.abstract.enRecent discoveries in two-dimensional magnetism have intensified the investigation of van der Waals magnetic materials and further improved our ability to tune their magnetic properties. Tunable magnetism has been widely studied in antiferromagnetic metal thiophosphates MPX3. Substitution of metal ions M has been adopted as an important technique to engineer the magnetism in MPX3. In this work, we have studied the previously unexplored chalcogen X substitutions in MPX3 (M=Mn/Ni; X=S/Se). We synthesized the single crystals of MnPS3−xSex (0≤x≤3) and NiPS3−xSex (0≤x≤1.3) and investigated the systematic evolution of the magnetism with varying x. Our study reveals the effective tuning of magnetic interactions and anisotropies in both MnPS3 and NiPS3 upon Se substitution. Such efficient engineering of the magnetism provides a suitable platform to understand the low-dimensional magnetism and develop future magnetic devices.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorPopielska, Magdalena
dc.contributor.authorHu, Jin
dc.contributor.authorAutieri, Carmine
dc.contributor.authorBishop, Samuel
dc.contributor.authorStephenson, Cory
dc.contributor.authorRybak, Milosz
dc.contributor.authorKotur, Kamila
dc.contributor.authorBasnet, Rabindra
dc.date.accessioned2024-01-24T20:47:38Z
dc.date.available2024-01-24T20:47:38Z
dc.date.copyright2022-06-23
dc.date.issued2022
dc.description.accesstimeAT_PUBLICATION
dc.description.financePublikacja bezkosztowa
dc.description.number2
dc.description.versionFINAL_PUBLISHED
dc.description.volume4
dc.identifier.doi10.1103/PHYSREVRESEARCH.4.023256
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/103706
dc.identifier.weblinkhttps://link.aps.org/article/10.1103/PhysRevResearch.4.023256
dc.languageeng
dc.pbn.affiliationphysical sciences
dc.relation.ispartofPhysical Review Research
dc.relation.pages023256-1-12
dc.rightsCC-BY
dc.sciencecloudnosend
dc.titleControlling magnetic exchange and anisotropy by nonmagnetic ligand substitution in layered MPX3 (M=Ni, Mn; X=S, Se)
dc.typeJournalArticle
dspace.entity.typePublication