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Light Emitting Spin Active Electronic States in Ultra-Thin Mn Doped CdSe Layered Nanosheets

cris.lastimport.scopus2024-02-12T19:52:41Z
dc.abstract.enThe layered nanosheets exhibit a variety of physical and optical properties originating from amalgamation of intra- and inter- layer electronic interactions, which makes them promising materials for advanced devices with varsatile controlling channels. In particular, the dilute magnetic semiconductor multilayered nanosheets have promising optical, electrical and magnetic properties that have been less explored so far. Here, the spin permissible optical properties from solvothermally grown Mn doped CdSe (thickness similar to 2.26 nm) multilayered nanosheets are reported on. The presence of multi-phase magnetic orderings with a sharp ferromagnetic transition at temperature similar to 48 K pertinent to the stabilization and co-existence of Mn2+ and Mn3+ based local phases have been observed from the (Cd, Mn) Se layered nanosheets corroborating to the x-ray absorption near edge structure, electron paramagnetic resonance, Raman scattering and magnetic measurements. The optical absorption and photoluminescence (PL) studies at room temperature affirm wide array of optical properties in the visible regime corresponding to the band edge and intriguing dopant-phase mediated spin approved transitions. The circularly polarized magneto-PL and life time analysis exhibits the spin-polarized fast radiative transitions confirming the presence of spin-active electronic states.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorJha, S. N.
dc.contributor.authorMohapatra, N.
dc.contributor.authorHalder, O.
dc.contributor.authorRath, S.
dc.contributor.authorRajput, P.
dc.contributor.authorPacuski, Wojciech
dc.contributor.authorSatpati, B.
dc.contributor.authorSuffczyński, Jan
dc.date.accessioned2024-01-25T05:10:49Z
dc.date.available2024-01-25T05:10:49Z
dc.date.issued2019
dc.description.financeNie dotyczy
dc.identifier.doi10.1038/S41598-019-38974-0
dc.identifier.issn2045-2322
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/111241
dc.languageeng
dc.pbn.affiliationphysical sciences
dc.relation.ispartofScientific Reports
dc.rightsClosedAccess
dc.sciencecloudnosend
dc.titleLight Emitting Spin Active Electronic States in Ultra-Thin Mn Doped CdSe Layered Nanosheets
dc.typeJournalArticle
dspace.entity.typePublication