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Impeded phase transition in 1T-TaS2: Thermoelectric fingerprint of long-lived mixed states

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dc.abstract.en1T-TaS2 is a material that belongs to the family of transition metal dichalcogenides and features a rich phase diagram including different charge density wave states. So far, most techniques used to study this material focus on either very local properties on the atomic scale or use global measurements of the whole sample like the electrical resistance. Here, we report on the influence of micrometer scale laser illumination on the global electric properties of a bulk sample. Thermoelectric effects are found to be responsible for a large electric response to the laser illumination. This effect is used to develop a method that allows to spatially map the thermoelectric properties of a 1T-TaS2 sample on the millimeter scale with micrometer resolution. We show that a specific temperature sweep can impede the phase transition, allowing to study long-lived mixed states, consisting of two phases. With this method we are able to image metastable states occurring in the transition between the nearly commensurate and commensurate charge density wave state in bulk 1T-TaS2 and compare the results to Raman spectroscopy.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorLutsyk, I.
dc.contributor.authorLacinska, E.
dc.contributor.authorBinder, Johannes
dc.contributor.authorStępniewski, Roman
dc.contributor.authorWysmołek, Andrzej
dc.contributor.authorRogala, Maciej
dc.contributor.authorKlusek, Zbigniew
dc.contributor.authorDąbrowski, Paweł
dc.contributor.authorLudwiczak, Katarzyna
dc.date.accessioned2024-01-25T03:57:20Z
dc.date.available2024-01-25T03:57:20Z
dc.date.issued2020
dc.description.financePublikacja bezkosztowa
dc.description.volume305
dc.identifier.doi10.1016/J.SSC.2019.113749
dc.identifier.issn0038-1098
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/109055
dc.identifier.weblinkhttp://dx.doi.org/10.1016/j.ssc.2019.113749
dc.languageeng
dc.pbn.affiliationphysical sciences
dc.relation.ispartofSolid State Communications
dc.relation.pages113749
dc.rightsClosedAccess
dc.sciencecloudnosend
dc.subject.enA. Transition metal dichalcogenides
dc.subject.enD. Phase transitions
dc.subject.enE. Raman spectroscopy
dc.subject.enE. Thermoelectric mapping
dc.subject.pldichalkogenki metali przejściowych
dc.subject.plprzejścia fazowe
dc.subject.plmapowanie termoelektryczne
dc.subject.plspektroskopia ramanowska
dc.titleImpeded phase transition in 1T-TaS2: Thermoelectric fingerprint of long-lived mixed states
dc.typeJournalArticle
dspace.entity.typePublication