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libcloudph++ 2.0: aqueous-phase chemistry extension of the particle-based cloud microphysics scheme

dc.abstract.enThis paper introduces a new scheme available in the library of algorithms for representing cloud microphysics in numerical models named libcloudph++. The scheme extends the particle-based microphysics scheme with a Monte Carlo coalescence available in libcloudph++ to the aqueous-phase chemical processes occurring within cloud droplets. The representation of chemical processes focuses on the aqueous-phase oxidation of the dissolved SO2 by O3 and H2O2. The particle-based microphysics and chemistry scheme allows for tracking of the changes in the cloud condensation nuclei (CCN) distribution caused by both collisions between cloud droplets and aqueous-phase oxidation. The scheme is implemented in C++ and equipped with bindings to Python. The scheme can be used on either a CPU or a GPU, and is distributed under the GPLv3 license. Here, the particle-based microphysics and chemistry scheme is tested in a simple 0-dimensional adiabatic parcel model and then used in a 2-dimensional prescribed flow framework. The results are discussed with a focus on changes to the CCN sizes and comparison with other model simulations discussed in the literature.
dc.affiliationUniwersytet Warszawski
dc.contributor.authorPawłowska, Hanna
dc.contributor.authorJaruga, Anna Barbara
dc.date.accessioned2024-01-25T05:09:35Z
dc.date.available2024-01-25T05:09:35Z
dc.date.issued2018
dc.description.financeNie dotyczy
dc.description.volume11
dc.identifier.doi10.5194/GMD-11-3623-2018
dc.identifier.issn1991-959X
dc.identifier.urihttps://repozytorium.uw.edu.pl//handle/item/111184
dc.identifier.weblinkhttps://www.geosci-model-dev.net/11/3623/2018/
dc.languageeng
dc.pbn.affiliationearth and related environmental sciences
dc.relation.ispartofGeoscientific Model Development
dc.relation.pages3623-3645
dc.rightsClosedAccess
dc.sciencecloudnosend
dc.titlelibcloudph++ 2.0: aqueous-phase chemistry extension of the particle-based cloud microphysics scheme
dc.typeJournalArticle
dspace.entity.typePublication